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NOx-reductive Perovskite catalysts for lean-burn engines

NOx-reductive Perovskite catalysts for lean-burn engines

          
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About the Book

In the present work Pd- and Rh- integrated perovskites are developed and characterized regarding the state of Pd and catalytic activity by means of microstructural and spectroscopic methods (XRD, SEM, TEM, XPS, and -SCR-NOx). Pd in the La- based perovskite partially displays a reversible diffusion mechanism under redox atmospheres at 600° C. These effects produce a self-regenerative mechanism at relatively high temperatures. Catalytic testing under model gas mixtures of powders and coatings of these perovskites proves the potential of these materials for effective NOx-reduction under lean conditions. Hydrogen provides the best NO- reduction results among the employed reducing agents (i.e. H2, C3H6, and C8H18). The Pd-integrated Perovskites display peak NO-conversions of 72 % and N2-selectivities of 72 % in the presence of H2O- vapour and CO2 at temperatures below 300°C. For instance, Ba- and Ce- substituted perovskites are also active for NO-reduction up to 400°C.


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Product Details
  • ISBN-13: 9783838111827
  • Publisher: Sudwestdeutscher Verlag Fur Hochschulschriften AG
  • Binding: Paperback
  • Language: English
  • Returnable: N
  • Spine Width: 10 mm
  • Width: 152 mm
  • ISBN-10: 3838111826
  • Publisher Date: 26 Oct 2009
  • Height: 229 mm
  • No of Pages: 164
  • Series Title: English
  • Weight: 250 gr


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